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中国物理学会期刊

扫描隧道显微镜中的量子相位研究

Probing Quantum Phase via Scanning Tunneling Microscopy

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  • 量子相位是刻画波函数性质与量子物态本质的重要物理量,蕴含着体系的几何、拓扑及多体关联等关键信息。长期以来,相位往往只能通过动量空间表征或宏观输运测量间接获取,难以在实空间中直接观测。近年来,扫描隧道显微镜(STM)及其谱学(STS)技术凭借原子级空间分辨率和对局域电子态的高度敏感性,为量子相位的实空间探测提供了新的实验途径。本文系统综述了基于STM的量子相位研究进展,重点介绍了四类代表性方法:通过局域干涉探测阿哈罗诺夫-玻姆效应的几何相位;借助缺陷诱导背散射与波前位错解析材料的拓扑相位;利用序参量分解重构魔角石墨烯等对称体系中的复相位结构;以及结合二维锁相技术研究非常规超导体中配对密度波与电荷密度波的相位纹理及拓扑缺陷。这些研究表明,STM能够将抽象的量子相位转化为可视化、可定量的实空间物理量,为理解拓扑物态、对称性破缺和电子关联提供了新的实验视角,也为未来相位工程和量子器件研究奠定了基础。

    Quantum phase is a fundamental physical quantity that characterizes the intrinsic properties of wave functions and quantum states, encoding critical information regarding the geometry, topology, and many-body correlations of a system. Traditionally, accessing this phase information has relied heavily on momentum-space probes or macroscopic transport measurements, making the direct visualization and quantification of quantum phases in real space a long-standing experimental challenge. In recent years, scanning tunneling microscopy/spectroscopy (STM/STS) have emerged as powerful platforms for directly probing quantum phases at the atomic scale, owing to their exceptional spatial resolution and sensitivity to local electronic states. This review summarizes the latest research progress of breakthroughs in STM-based quantum phase research, with a specific focus on four highly innovative methodologies and their corresponding experimental results.
    We first discuss the probing of geometric phases via local Aharonov-Bohm (AB) interferometry, where nanoscale real-space interferometers constructed with STM enable direct resolution of coherent local density of states (LDOS) oscillations driven by external magnetic fluxes, allowing quantitative extraction of geometric phases. Next, we examine the resolution of topological phases through defect-induced backscattering; by carefully analyzing quasiparticle interference and associated wavefront dislocations around atomic defects, this approach enables direct extraction of topological invariants, such as winding numbers, and Berry phases without the need for an external magnetic field. We then describe the reconstruction of complex phase structures via order-parameter decomposition, highlighting advanced spatial decomposition techniques applied to strongly correlated and highly symmetric systems, such as magic-angle twisted bilayer graphene, which successfully disentangle intertwined orders and provide crucial experimental criteria for identifying microscopic ground states. Furthermore, we review the investigation of phase textures and topological defects using 2D lock-in techniques; applied to unconventional superconductors, these spatial filtering methods enable high-precision mapping of phase modulations in pair density wave (PDW) and charge density wave (CDW), and successfully visualize topological defects such as phase jumps, vortices, and half-dislocations. These transformative advances demonstrate that STM and associated analytical techniques effectively translate abstract mathematical quantum phases into visualizable, quantifiable real-space observables. This not only offers profound new experimental perspectives for decoding topological states of matter, symmetry breaking, and complex electronic correlations, but also lays a solid foundation for future phase engineering and the development of next-generation quantum devices.

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