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中国物理学会期刊

桌面式极紫外高次谐波光源的产生及模拟

Generation and Simulation of Tabletop Extreme Ultraviolet High-Order Harmonics

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  • 极紫外高次谐波光源是探究超快电子动力学过程的重要工具,在阿秒及飞秒物理、化学等研究中得到了广泛关注。本文围绕桌面式高次谐波产生过程的实验特性及其物理机制开展了实验与数值模拟研究。通过调控气体压强和驱动激光功率,在有限相互作用长度条件下实现了有效的宏观相位匹配,显著增强了谐波辐射强度,获得了光子能量覆盖20-40 eV的极紫外高次谐波辐射。结合气体介质中谐波场的宏观传播模型,对高次谐波的产生过程进行了模拟,通过对计算与实验观测结果比较,揭示了谐波增强的物理机制,表明该差分有限气室结构能够实现可重复的XUV谐波输出。上述研究为桌面式极紫外高次谐波光源在超快物理、化学研究中的推广提供了实验与理论依据。

    Tabletop extreme ultraviolet (XUV) sources based on high-order harmonic generation (HHG) play a crucial role in ultrafast and attosecond science. In this work, a compact HHG system employing a differentially finite gas cell is developed, and XUV harmonic generation under a limited interaction length is systematically investigated.
    Driven by an 800 nm titanium–sapphire femtosecond laser, efficient macroscopic phase matching is achieved through coordinated optimization of gas species, gas pressure, and driving laser power. Using krypton and xenon as target gases, stable XUV radiation covering photon energies of 20–40 eV is obtained. The harmonic yield exhibits a clear dependence on gas pressure and laser intensity. It is found that, in low-ionization-potential gases, increased ionization enhances plasma dispersion and aggravates phase mismatch, limiting further growth of the harmonic intensity.
    Numerical simulations based on a macroscopic propagation model, incorporating neutral-gas dispersion, plasma dispersion, Gouy phase shift, and dipole phase, reveal the formation of a localized phase-matching region near the pinhole. This localized condition facilitates the coherent buildup of harmonic emission and reduces reabsorption. The simulated spectra agree well with experimental results, validating the model. The proposed scheme provides a simple and robust approach for generating stable and reproducible tabletop XUV sources, offering potential applications in ultrafast spectroscopy.

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