搜索

x
中国物理学会期刊

基于白光中子源的159Tb(n,γ)反应截面测量及共振参数分析

Measurement of the 159Tb(n,γ) Reaction Cross Section and Resonance Parameter Analysis Based on the White Neutron Source CSNS Back-n

PDF
导出引用
  • 铽(Tb)(n,γ)反应截面是核工程计算与恒星s过程研究中的重要基础核数据,在反应堆活化分析及稀土区丰度计算中具有重要作用。该反应的实验研究主要包括基于反应堆或加速器中子源的飞行时间法测量以及活化法测量等,集中在热中子附近和MeV能区,在可分辨共振区,已有实验数据仍较为有限,对该能区的高精度测量有助于完善相关共振参数的信息。故利用全吸收型伽马探测装置(Gamma Total Absorption Facility,GTAF),基于中国散裂中子源(CSNS)反角白光中子(Back-n)束线,对159Tb (n,γ)反应截面进行了在线测量。实验采用飞行时间(TOF)方法确定中子能量,通过死时间修正、脉冲形状甄别、多重性筛选和加和能量判选、本底扣除等处理后提取了中子俘获产额。随后使用SAMMY程序通过R矩阵分析提取了1–100 eV的共振参数并重构了该能区的反应截面,为现有核数据评价提供了新的参考,同时也为相关核天体物理计算和核工程应用提供了可靠的实验基础。

    Neutron capture on deformed rare-earth nuclei provides stringent tests of nuclear reaction models and constitutes a key benchmark for both nuclear data evaluation and s-process nucleosynthesis studies. As a stable odd-A rare-earth nucleus with a pronounced deformed structure, 159Tb plays an important role in reactor-related calculations, activation analysis, nuclear data evaluation, and s-process nucleosynthesis in the rare-earth mass region. Although previous measurements have been performed at thermal and MeV neutron energies, experimental data in the eV to several hundred eV region remain scarce, and independent constraints on resonance parameters are still limited. To provide independent experimental constraints in this energy region, the 159Tb(n,γ) reaction cross section is measured at the Back-n white neutron beam line of the China Spallation Neutron Source (CSNS) using the Gamma Total Absorption Facility (GTAF). The incident neutron energy is determined by the time-of-flight method over a wide white neutron spectrum. Capture events are identified by applying summed-energy window selection, crystal multiplicity gating, and pulse-shape discrimination to suppress background contributions. Dead-time correction is performed to account for the high instantaneous counting rate of the detection system. Background components are evaluated and subtracted using dedicated measurements with natC and empty samples, leading to the net capture yield spectrum. Based on these procedures, the experimental cross section is obtained over the 1–1000 eV energy range.
    An R-matrix analysis was performed using the SAMMY code to extract resonance parameters in the resolved resonance region (1–100 eV). The extracted resonance energies and widths well reproduce the main resonance structures and are consistent with the ENDF/B-VIII.0 evaluation within uncertainties, with no indication of systematic bias. Comparison with ENDF/B-VIII.0, JEFF-4.0, JENDL-5 and BROND-3.1 shows overall consistency in the major resonance structures and energy dependence, although some local discrepancies remain in weak or complex regions. Several weak structures are observed in the experimental spectrum; although they may suggest resonance-like features, contributions from sample impurities and neutron-beam-related effects and local analysis sensitivity cannot be excluded, and a definitive interpretation requires further study. The present work provides both experimental cross sections in the 1–1000 eV region and independently extracted resonance parameters in the 1–100 eV region, thereby strengthening the experimental basis for resonance-region nuclear data of 159Tb. The present measurement provides independent experimental constraints on neutron capture in a deformed rare-earth nucleus and establishes 159Tb as a rare-earth benchmark for resonance-region nuclear data, contributing to improved reliability of evaluated libraries for nuclear astrophysics and reactor-related applications.

    目录

    返回文章
    返回