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2024, 73 (19): 190101.
Abstract +
Intrinsic mechanism of influence of channel blocking and noise on response state of multicompartmental neurons
Chen Yu-Wei, Fang Tao, Fan Ying-Le, She Qing-Shan
2024, 73 (19): 190501.
Abstract +
The fine structure of multi-compartment neurons can simultaneously capture both temporal and spatial characteristics, offering rich responses and intrinsic mechanisms. However, current studies of the effects of channel blockage and noise on neuronal response states are mainly limited to single-compartment neurons. This study introduces an analytical method to explore theintrinsic mechanism of channel blockage and noise effects on the response states of multi-compartment neurons, by using the smooth Pinsky-Rinzel two-compartment neuron model as a case study. Potassium, sodium, and calcium ion channel blockage coefficient are separately introduced to develop a smooth Pinsky-Rinzel neuron model with ion channel blockage. Methods such as single-parameter bifurcation analysis, double-parameter bifurcation analysis, coefficient of variation, and frequency characteristics analysis are utilized to examine the effects of various ion channel blockages on neuronal response states. Additionally, smooth Pinsky-Rinzel neuron Subunit noise model and conductance noise model are constructed to investigate their response characteristics by using interspike interval analysis and coefficient of variation indicators. Subthreshold stimulation is used to explore the presence of stochastic resonance phenomena. Single-parameter bifurcation analysis of the ion channel blockage model elucidates the dynamic processes of two torus bifurcations and limit point bifurcations in Pinsky-Rinzel neuron firing under potassium ion blocking. Double-parameter bifurcation analysis reveals a nearly linear increase in the Hopf bifurcation node of potassium ions with input current, whereas sodium ions exhibit a two-stage pattern of linear decline followed by exponential rise. The analysis of average firing frequency and coefficient of variation indicates that the moderate potassium channel blockage promotes firing, sodium channel blockage inhibits firing, and calcium channel blockage shows the complex characteristics but mainly promotes firing. Subthreshold stimulation of the channel noise model demonstrates the stochastic resonance phenomena in both models, accompanied by more intense chaotic firing, highlighting the positive role of noise in neural signal transmission. The interspike interval and coefficient of variation indicators show consistent variation levels for both noise models, with the conductance model displaying greater sensitivity to membrane area and stronger encoding capabilities. This study analyzes the general frequency characteristics of potassium and sodium ions in a multi-compartment neuron model through ion channel blocking model, providing special insights into the unique role of calcium ions. Further, the study explores stochastic resonance by using ion channel noise model, supporting the theory of noise-enhanced signal processing and offering new perspectives and tools for future studying complex information encoding in neural systems. By constructing an ion channel blockage model, the effects of potassium and sodium ions on the frequency characteristics of multi-compartment neurons are analyzed and the special influences of calcium ions are revealed. Using the ion channel noise model, the stochastic resonance is investigated, supporting the theory that the noise enhances signal processing. This research offers a new perspective and tool for studying the complex information encoding in neural systems.
Algorithm of reconstrucing temperature correction curve of digital thermometer based on pseudo inverse method
Kang Zhe-Ming, Ji Jin-Long, Kang Pin-Chun, Liu Jun-Jian, Lü Yi-Hui, Guo Lu-Qing
2024, 73 (19): 190701.
Abstract +
At present, high-precision digital thermometers based on industrial platinum resistance have become a popular research direction and are widely used in environmental monitoring, medical health, industrial automation and other fields. However, due to the influence of materials and manufacturing processes, the measurement accuracy is average. With the increase of service life, it is inevitable that the temperature measurement deviation will be caused by the drift of the resistance value. The algorithm of correcting temperature is an effective method to improve the measurement accuracy of digital thermometers. Traditional compensation function correction algorithms such as polynomial fitting and B-spline fitting have good correction effect, but the problems of resistance drift cannot be solved. The segmented linear correction algorithm is simple and easy to implemente, but it requires multi-point temperature measurements. Because of the nonlinear changes of the temperature correction curve, the correction effect is average, which limits its correction accuracy and universality. Therefore, we proposenalgorithm of reconstructing temperature correction curve based on the pseudo inverse method. Firstly, the reconstruction matrix is built by using the original data and multiple characteristic temperature points. Then, the complete temperature correction curve is reconstructed by the characteristic temperature points to be reconstructed and the reconstruction matrix. Finally, the reconstructed temperature correction curve is automatically included in the sample database, which improves the diversity of samples and the correction accuracy of the algorithm. Experimental results show that the proposed algorithm has a better correction effect on nonlinear changes and drifts of the temperature correction curve. And the proposed algorithm is less affected by the number of characteristic temperature points and the selection combination. The complete temperature correction curve is well reconstructed by collecting only 4 characteristic temperature points. Therefore, the proposed algorithm can provide the effective support for improving the measurement accuracy of digital thermometer.
Optimization of electrical properties and radio frequency applications of GeTe thin film
Shuai Chen-Yang, Zheng Yue-Jun, Chen Qiang, Ma Yan-Li, Fu Yun-Qi
2024, 73 (19): 190702.
Abstract +
GeTe belongs to a chalcogenide phase change material, which can dynamically achieve reversible switching between the crystalline state of low resistivity and the amorphous state of high resistivity by utilizing the thermally induced phase change characteristics. The GeTe is an important functional material in the fields of memristors and nonvolatile radio frequency (RF) switches. For RF switch applications, this paper focuses on optimizing the electrical performance of GeTe thin films prepared by magnetron sputtering. By comprehensively analyzing the effects of substrate materials, sputtering conditions, and annealing conditions on the resistivity of crystalline GeTe films, effective conditions for preparing low resistivity GeTe films are explored. Fig. (a) shows that compared with the GeTe film on a SiO2substrate, the film on an Al2O3substrate can obtain higher crystallinity and lower resistivity. For the deposition power and pressure shown in Fig. (b), the combination of medium power (50–80 W) and low pressure (2–3 mTorr) is beneficial for low crystalline resistivity of GeTe film. Additionally, Fig. (c) shows that higher annealing temperature (350–400 ℃) can realize lower film resistivity. Finally, the experimental results show that the lowest crystalline resistivity of the prepared GeTe thin film reaches 3.6×10–6Ω·m, and the resistance ratio is more than 106. Based on rectangular chips of GeTe film, a parallel millimeter-wave switch with zero static power is also constructed. As shown in Fig. (d), the insertion loss is less than 2.4 dB, and the isolation is greater than 19 dB in a 1–40 GHz frequency band, demonstrating the potential application of GeTe thin films in the field of broadband high-performance discrete nonvolatile RF switches.
Hefei Advanced Light Facility: Empowering research of correlated electron systems
Sun Zhe, Shen Da-Wei, Luo Zhen-Lin, Yan Wen-Sheng
2024, 73 (19): 190703.
Abstract +
The Hefei Advanced Light Facility is the fourth-generation diffraction-limited storage ring light source, scheduled to begin operation in 2028. With its high-brightness and highly coherent X-rays, it will break through the current spatiotemporal resolution bottlenecks of X-ray techniques in studying correlated electron systems, providing crucial information for understanding the nature and microscopic origins of novel physical properties in these materials. This article introduces the main scientific goals and technical advantages of the Hefei Advanced Light Facility, focusing on the application perspectives of advanced technologies such as angle-resolved photoemission spectroscopy, magnetic circular dichroism, coherent X-ray scattering, and coherent X-ray imaging in researches of quantum materials and correlated electron systems. These techniques will enable the detailed analysis of the distribution and dynamics of electronic/spin/orbital states, reveal various novel quantum phenomena, and elucidate the fluctuations of order parameters in correlated electron systems. The completion of the Hefei Advanced Light Facility will provide advanced technical supports for decoding complex quantum states and non-equilibrium properties, ultimately promoting the application of quantum materials and correlated electron systems in frontier fields such as energy and information.
Research on vibrational features of CL-20/MTNP cocrystal by terahertz spectroscopy
Liu Quan-Cheng, Yang Fu, Zhang Qi, Duan Yong-Wei, Deng Hu, Shang Li-Ping
2024, 73 (19): 193201.
Abstract +
Cocrystals represent an effective method to manipulate the physicochemical properties of materials at a molecular level. However, understanding the relationship between their complex crystal structures and macroscopic properties is a challenge. In this paper, by using terahertz (THz) spectroscopy to characterize non-covalent interactions within crystals, the THz vibrational spectra of the CL-20/MTNP cocrystal are studied. Firstly, the THz spectra of CL-20, MTNP, and the CL-20/MTNP cocrystal are measured at room temperature. Both absorption positions and intensities of the cocrystals differ from those of their original components, confirming the unique advantage of terahertz spectroscopy in cocrystal identification. Secondly, the THz vibrational features of the three materials are calculated based on density functional theory (DFT). Then, the experimental absorptions are matched with the calculated vibrations. Furthermore, a vibrational decomposition method is employed to decompose the molecular vibrations into intermolecular and intramolecular vibrations. The vibrational variations of the cocrystal compared with its original components are analyzed. The results reveal that in the cocrystal, the intermolecular vibrational modes of both CL-20 and MTNP molecules have changed compared with their raw materials. This indicates that the non-covalent interactions in the cocrystal have changed the original intermolecular interactions of these molecules. Consequently, this enhancement promotes the heat transfer between MTNP and CL-20 molecules, thereby improving the thermal stability of the cocrystal. These findings in this study demonstrate that the THz vibrational spectroscopy technology helps establish a relationship between the molecular structure of cocrystal and its macroscopic properties. This research contributes to deepening our understanding of cocrystal systems and opens up a new way for designing and optimizing materials.
Geometry and electronic structures of rare earth-doped boron-based clusters $ {\text{REB}}_n^ - $ (RE = La, Sc;n= 6, 8)
Chen Zi-Jun, Li Hui-Fang, Xie Zhen-Ming, Zhang Yong-Hang, Zheng Hao, Jiang Kai-Le, Zhang Bo, Zhang Jia-Ming, Wang Huai-Qian
2024, 73 (19): 193601.
Abstract +
Rare earth doped boron clusters have attracted much attention due to their special optical, electrical and magnetic properties. The geometric structures, stability, electronic properties and aromaticity of negative rare earth doped boron clusters $ {\text{REB}}_n^ - $ (RE = La, Sc;n= 6, 8) are investigated with the artificial bee colony algorithm combined with density functional theory calculations at the PBE0/RE/SDD//B/6-311+G* level of theory. Calculations show that the ground state structures of $ {\text{REB}}_n^ - $ (RE = La, Sc;n= 6, 8) are all ofC2symmetry, and the doped lanthanide atom is located in a “boat-shaped” structure at the top center. By comparing with the experimental photoelectron spectra, it is confirmed that the ground state structure of $ {\text{LaB}}_{8}^ - $ is a “zither-like” three-dimensional structure, and the ground state structure of $ {\text{ScB}}_{8}^ - $ is an “umbrella” structure withC7Vsymmetry formed by the scandium atom at the “umbrella handle”. The electron localization between RE—B is not as good as that between B—B. The simulated photoelectron spectra have similar spectral characteristics to the experimental results. The lowest energy structures of $ {\text{LaB}}_{6}^ - $ and $ {\text{ScB}}_{6}^ - $ areσ-π double aromatic clusters, and the structures exhibit aromaticity. The density of states of low-energy isomers shows that the open shell $ {\text{ScB}}_{8}^ - $ density of states spectrum exhibits spin polarization phenomenon, which is expected to assemble magnetic material components. These studies contribute to understanding the evolution of structure and properties of nanomaterials, and provide important theoretical support for designing nanomaterials with practical value.
Advances in free-electron-laser based scattering techniques and spectroscopic methods
Zhong Yin-Peng, Yang Xia
2024, 73 (19): 194101.
Abstract +
In 2005, the FLASH soft X-ray free-electron laser (FEL) in Hamburg, Germany, achieved its first lasing, which began an intensive phase of global FEL construction. Subsequently, the United States, Japan, South Korea, China, Italy, and Switzerland all began building such photon facilities. Recently, the new generation of FEL has started to utilize superconducting acceleration technology to achieve high-repetition-rate pulse output, thereby improving experimental efficiency. Currently completed facility is the European XFEL, ongoing constructions are the LCLS-II in the United States and the SHINE facility in Shanghai, and the facility in preparation is the Shenzhen superconducting soft X-ray free-electron laser (S 3FEL). These FEL facilities generate coherent and tunable ultrashort pulses ranging from the extreme ultraviolet to hard X-ray spectrum, which advances the FEL-based scattering techniques such as ultrafast X-ray scattering, spectroscopy, and X-ray nonlinear optics, thereby transforming the way we study correlated quantum materials on an ultrafast timescale. The self-amplified spontaneous emission (SASE) process in FEL leads to timing jitter between FEL pulses and the synchronized pump laser, influencing the accuracy of ultrafast time-resolved measurements. To address this issue, timing tools have been developed to measure these jitters and reindexed each pump-probe signal after measurement. This success enables ultrafast X-ray diffraction (UXRD) to be first realized, and a systematic study of Peierls distorted materials is demonstrated. In addition, the high flux of FEL pulses enables Fourier transform inelastic X-ray scattering (FT-IXS) method, which can extract the phonon dispersion curve of the entire Brillouin zone by performing the Fourier transform on the measured momentum dependent coherent phonon scattering signals, even when the system is in a non-equilibrium state. The UXRD is typically used to study ultrafast lattice dynamics, which requires hard X-ray wavelengths. In contrast, time resolved resonant elastic X-ray scattering (tr-REXS) in the soft X-ray regime has become a standard method of investigating nano-sized charge and spin orders in correlated quantum materials on an ultrafast time scale. In correlated quantum materials, the interplay between electron dynamics and lattice dynamics represents another important research direction. In addition to Zhi-Xun Shen's successful demonstration of the combined tr-ARPES and UXRD method at SLAC, this paper also reports the attempts to integrate UXRD with resonant X-ray emission spectroscopy (RXES) for the simultaneous measurement of electronic and lattice dynamics. Resonant inelastic X-ray scattering (RIXS) is a powerful tool for studying elementary and collective excitations in correlated quantum materials. However, in FEL-based soft X-ray spectroscopy, the wavefront tilt introduced by the widely used grating monochromators inevitably stretches the FEL pulses, which degrades the time resolution. Therefore, the new design at FEL beamlines adopts low line density gratings with long exit arms to reduce pulse stretch and achieve relatively high energy resolution. For example, the Heisenberg-RIXS instrument at the European XFEL achieves an energy resolution of 92 meV at the Cu L 3edge and approximately 150 fs time resolution. In recent years, scientists at SwissFEL’s Furka station have drawn inspiration from femtosecond optical covariance spectroscopy to propose a new method of generating two-dimensional time-resolved resonant inelastic X-ray scattering (2D tr-RIXS) spectra. This method involves real-time detection of single-shot FEL incident and scattered spectra, followed by deconvolution calculation to avoid photon waste and wavefront tilt caused by monochromator slits. The SQS experimental station at European XFEL, built in 2023, features a 1D-XUV spectrometer that utilizes subtle variations in photon energy absorption across the sample to induce spatial energy dispersion. Using Wolter mirrors, it directly images spatially resolved fluorescence emission from the sample onto the detector to generate 2D tr-RIXS spectra without the need for deconvolution. However, this design is limited to specific samples. Currently, the S 3FEL under designing has a novel 2D tr-RIXS instrument that uses an upstream low line density grating monochromator to generate spatial dispersion of the beam spot, allowing the full bandwidth of SASE to project spatially dispersed photon energy onto the sample. Subsequently, an optical design similar to the 1D-XUV spectrometer will be employed to achieve 2D tr-RIXS spectra, thereby expanding the applicability beyond specific liquid samples. These new instruments are designed to minimize pulse elongation by fully utilizing SASE’s full bandwidth, approaching Fourier-transform-limited RIXS spectra in both time and energy resolution. Nonlinear X-ray optical techniques, such as sum-frequency generation (SFG) and second-harmonic generation, are adapting to X-ray wavelengths and opening up new avenues for detecting elementary excitations. The X-ray transient grating spectroscopy extends its capabilities to studying charge transport and spin dynamics on an ultrafast timescale. The future development of these scattering methods provides unique opportunities for detecting dynamical events in various systems, including surface and interface processes, chirality, nanoscale transport, and so-called multidimensional core-level spectroscopy.
Attosecond delay locking of large arm pump-probe system
Wang Ke-Jian, Teng Hao, Xing Xiao-Wei, Dong Shuo, Cao Kai-Qiang, Jiang Yu-Jiao, Zhao Kun, Zhu Jiang-Feng, Liu Wen-Jun, Wei Zhi-Yi
2024, 73 (19): 194201.
Abstract +
With the development of ultrafast science and attosecond laser technology, the pump-probe system based on isolated attosecond laser pulses is a key to attosecond science, which will be used to study electronic dynamics on an attosecond time-scale. To obtain stable and reliable signals, it is necessary to ensure ultra-stable and ultra-accurate synchronization. Any timing jitter can cause signal to disperse or get buryied in noise, making it impossible to obtain the true physical mechanism. Based on the above, the delay between pump laser pulse and probe laser pulse must be controlled with an attosecond time resolution. In this work, a dual-layer system is developed to achieve high-precision synchronization locking. To ensure that both layers have the same time jitter, we design an adapter to secure the elements placed during installation. Timing jitter is obtained by shaking interference fringes through fast Fourier transformation, and can be calculated in several ms. Then error signals are fed back to the PZT stage in order to compensate for real-time optical path drift. Through such a design, a time-delay accuracy of 7.64 as to 15.53 as is realized, which is linearly related to the interferometer arm length ranging from 1 m to 5 m, with anR2of 0.96. Moreover, the error between the experimental result of arm length of 8 m and 10 m and the result fitted with the above data is less than 3 as. These results show that using a small interferometer can achieve the fast detection of the time-delay accuracy of long-arm attosecond pump-probe detection system in large scientific instrument, which is of great significance in guiding ther applications such as in non-collinear attosecond streaking spectroscopy, time-resolved photoelectron spectroscopy, and coherent synthesis.
Over-30-GeV intense laser phase-locked direct electron acceleration
Zhu Han-Chen, Zhou Chu-Liang, Li Xiao-Feng, Tian Ye, Li Ru-Xin
2024, 73 (19): 195201.
Abstract +
When an intense laser obliquely irradiates a solid, a pre-pulse will first ionize the solid surface, followed by the main pulse interacting with the plasma and ultimately being reflected by the plasma. Simultaneously, certain electrons within the plasma will be trapped in the accelerating phase of the laser field, subsequently gaining effective acceleration within the field, this phenomenon is known as phase-locked electron acceleration. Given the current intense lasers' electric field intensity nearing the TV/m range, electrons could potentially acquire energy levels on the order of hundreds of GeV or even TeV, provided they stay in the accelerating phase of the laser field long enough. Here, we initially use PIC (Particle-in-Cell) simulations to simulate the interaction process between laser pulses and plasma, thereby obtaining the properties of phase-locked electrons. In order to reduce computational demands, we turn to use a three-dimensional (3D) test particle model to calculate the subsequent interactions of these electrons with the reflected laser field. By this model, we obtain the data of the locked-phase electrons after having interacted with the reflected laser (Fig. (a)). Furthermore, we use this model to calculate the dynamical behavior of electrons under different initial conditions (Fig. (b)). Under the laser intensity of $ {a}_{0}=350 $ ( $ {a}_{0} $ is the normalized laser vector potential), the energy of the electrons directly accelerated by the laser is enhanced to 32 GeV. In contrast, under the same laser intensity, the energy of the electrons accelerated by ponderomotive force is only 0.35 GeV. The research findings indicate that the strong laser with peak power around 10 PW can directly accelerate electrons to approximately 30 GeV. Additionally, this study outlines the optimal initial conditions for injecting electrons into the laser field and the final electron energy within the phase-locked acceleration mechanism, thereby establishing a calibration relationship with the laser field intensity. Given the continual enhancement of laser intensity and the potential application of the laser phase-locked electron acceleration mechanism to positron acceleration, this research holds promise for its implementation in fields such as miniaturized positron-electron colliders and high-energy gamma-ray sources.
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